Gargamel

Hank Azaria

Acting

Patrick Winslow

Neil Patrick Harris

Acting

Grace Winslow

Jayma Mays

Acting

Papa Smurf (voice)

Jonathan Winters

Acting

Smurfette (voice)

Katy Perry

Acting

Clumsy Smurf (voice)

Anton Yelchin

Acting

Odile Anjelou

Sofía Vergara

Acting

Henri

Tim Gunn

Acting

Azrael (voice)

Frank Welker

Acting

Model

Madison McKinley

Acting

Model

Meg Phillips

Acting

Cabbie

Mahadeo Shivraj

Acting

Newscaster

Julie Chang

Camera

Bluetooth Businessman

Mark Doherty

Acting

Young Woman

Minglie Chen

Acting

Guy in Plaid Shirt

Sean Kenin

Acting

Bum

Victor Pagan

Acting

Anjelou Employee

Adria Baratta

Acting

Odile's Mother

Paula Pizzi

Acting

Waiter

Andrew Sellon

Acting

Little Sister

Julianna Rigoglioso

Acting

Blonde Sister

Daria Rae Figlo

Acting

Toy Salesperson

Bradley Gosnell

Acting

Toy Store Parent

Heidi Armbruster

Acting

Toy Store Parent

Finnerty Steeves

Acting

Parent with Girls

John Speredakos

Acting

Kicking Girl

Skai Jackson

Acting

Skateboard Kid

Alex Hall

Acting

Skateboard Kid

Eric Redgate

Acting

FAO Custodian

Jojo Gonzalez

Acting

Cop

Scott Dillin

Acting

Cop

Tyree Michael Simpson

Acting

Inmate Bubba

Sean Ringgold

Acting

Bubba's Inmate Friend

Mario D'Leon

Acting

Party Guest

Liz Smith

Acting

Party Guest

Tom Colicchio

Acting

Party Guest

Michael Musto

Acting

Party Guest

Joan Rivers

Acting

Party Guest

Olivia Palermo

Acting

Party Guest

Julia Enescu

Production

Party Guest

Lauren Waggoner

Acting

Azrael

Mr. Krinkle

Acting

Elway

Hank

Acting

Gutsy Smurf (voice)

Alan Cumming

Acting

Brainy Smurf (voice)

Fred Armisen

Acting

Grouchy Smurf (voice)

George López

Acting

Greedy Smurf (voice)

Kenan Thompson

Acting

Handy Smurf (voice)

Jeff Foxworthy

Acting

Vanity Smurf (voice)

John Oliver

Acting

Chef Smurf (voice)

Wolfgang Puck

Acting

Hefty Smurf (voice)

Gary Basaraba

Acting

Jokey Smurf (voice)

Paul Reubens

Acting

Baker Smurf (voice)

B. J. Novak

Acting

Narrator Smurf (voice)

Tom Kane

Acting

Crazy Smurf (Voice)

John Kassir

Acting

Farmer Smurf (voice)

Joel McCrary

Acting

Mother of Girl in Store (uncredited)

Mary McGloin

Acting