Steve Rogers / Captain America

Chris Evans

Acting

Nick Fury

Samuel L. Jackson

Acting

Natasha Romanoff / Black Widow

Scarlett Johansson

Acting

Alexander Pierce

Robert Redford

Acting

Bucky Barnes / Winter Soldier

Sebastian Stan

Acting

Sam Wilson / Falcon

Anthony Mackie

Acting

Maria Hill

Cobie Smulders

Acting

Brock Rumlow

Frank Grillo

Acting

Jasper Sitwell

Maximiliano Hernández

Acting

Kate / Agent 13

Emily VanCamp

Acting

Peggy Carter

Hayley Atwell

Acting

Dr. Arnim Zola

Toby Jones

Acting

Smithsonian Guard

Stan Lee

Writing

Jack Rollins

Callan Mulvey

Acting

Councilwoman Hawley

Jenny Agutter

Acting

Councilman Singh

Bernard White

Acting

Councilman Rockwell

Alan Dale

Acting

Councilman Yen

Ng Chin Han

Acting

Senator Stern

Garry Shandling

Acting

Georges Batroc

Georges St-Pierre

Acting

French Pirate #1

Salvator Xuereb

Acting

French Pirate #2

Brian Duffy

Crew

Engine Pirate

Zack Duhame

Crew

French Radio Pirate

Adetokumboh M'Cormack

Acting

Skinny Steve

Christopher George Sarris

Acting

Launch Tech #1

Aaron Himelstein

Acting

Launch Tech #2

Allan Chanes

Acting

Dr. Fine

Joe Russo

Directing

SHIELD Interrogator #1

Christopher Markus

Writing

SHIELD Interrogator #2

Stephen McFeely

Writing

Scientist #1

Pat Healy

Acting

Scientist #2

Ed Brubaker

Writing

Apple Employee

D.C. Pierson

Acting

Com Tech #1

Danny Pudi

Acting

Com Tech #2

Bernie Zilinskas

Acting

Renata

Branka Katić

Acting

Garcia

Angela Russo-Otstot

Production

Charlie XO

Jon Sklaroff

Acting

Charlie Weapons Tech

Chad Todhunter

Acting

SHIELD Tech

Abigail Marlowe

Acting

Lead SHIELD Pilot

Jeremy Maxwell

Acting

Senior SHIELD Agent

Emerson Brooks

Acting

SHIELD Agent

Evan Parke

Acting

Strike SGT. #1

Ricardo Chacon

Acting

Strike SGT. #2

Griffin M. Allen

Acting

Strike Agent

Ann Russo

Acting

Strike Agent

Joe Rosalina

Acting

Strike Agent

Michael Debeljak

Acting

Strike Agent

Eddie J. Fernandez

Crew

25ᵗʰ Floor Strike Agent

Jody Hart

Acting

Scudder

Steven Culp

Acting

Human Resources Executive

Derek Hughes

Acting

Doctor

Wendy Hoopes

Acting

Lead EMT

Ethan Rains

Acting

CIA Instructor

Dominic Rains

Acting

Capitol Hill Police

Charles Wittman

Acting

Capitol Hill Police

Andy Martinez, Jr.

Acting

FBI Agent

Michael De Geus

Acting

FBI Agent

Terence O'Rourke

Acting

Committee Member

Anne Grimenstein

Acting

Little Boy in the Smithsonian

Dante Rosalina

Acting

Fury Car Voice (voice)

Robert Clotworthy

Acting

SHIELD Computer (voice)

June Christopher

Acting

The Smithsonian Narrator (voice)

Gary Sinise

Acting

Dr. List (uncredited)

Henry Goodman

Acting

SHIELD Agent (uncredited)

Dean Barlage

Acting

Museum Visitor (uncredited)

Joel Thingvall

Acting

Baron Wolfgang von Strucker (uncredited)

Thomas Kretschmann

Acting

Wanda Maximoff / Scarlet Witch (uncredited)

Elizabeth Olsen

Acting

Committee General (uncredited)

Nestor Serrano

Acting

Pietro Maximoff / Quicksilver (uncredited)

Aaron Taylor-Johnson

Acting

Man on Escalator in Museum (uncredited)

Joss Whedon

Writing

Smithsonian Museum Visitor

James Lewis

Acting

S.H.I.E.L.D. Strike Agent (uncredited)

Josh Heileman

Acting

Pedestrian (uncredited)

Dominique Henderson

Acting